You can block a phone number on iPhone directly from the Phone app. Or go to Settings>Phone>Block>Add New and add the phone number you want to block to the blocked list. Here's a more detailed guide on blocking a number on iPhone: How to Block Numbers on iPhone and Find Blocked Numbers on iPhone
You can block any number on your iPhone by just installing an app called "iBlacklist"
In the app you have many options, and with them there's an option of blocking a cellphone number.
You
go to Blacklists - General BL. There you have '+' in upper right
corner. From there you can add the number you want from contacts, recent
calls and messages or write it yourself.
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